Break-in he'd orchestrated in part of Merseyside (10)
I believe the answer is:
birkenhead
'part of merseyside' is the definition.
The definition suggests a singular noun which matches the answer.
'break-in he'd orchestrated' is the wordplay.
'orchestrated' is an anagram indicator (arranged, as music).
'break'+'in'+'hed'='breakinhed'
'breakinhed' is an anagram of 'BIRKENHEAD'.
'in' is the link.
Can you help me to learn more?
(Another definition for birkenhead that I've seen is " Port, say".)
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