Crossword Genius

Group of Outer Hebrides islands, at least nine of which are populated (4)

Ross

I believe the answer is:

uist

(Other definitions for uist that I've seen before include "North and South islands of the Outer Hebrides" , "Hebridean islands, North and South ____" , "Hebridean island" .)

I've seen this clue in The Sunday Times and The Times.
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